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The Soundtrackcollector database contains:
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A search for 'The Man From U.N.C.L.E' gave the following results:

6 matches in labels:
  1. Man From U.N.C.L.E., The (RCA Victor LSP 3574)
    Original Release Title: More Music From The Man From U.N.C.L.E.
    Arranged and conducted by Hugo Montenegro.
  2. Man From U.N.C.L.E., The (RCA/BMG Music Spain 74321637062)
    Original Release Title: More Music From The Man From U.N.C.L.E.
  3. Man From U.N.C.L.E., The (Film Score Monthly FSMCD Vol. 6, No. 17)
    Original Release Title: Man From U.N.C.L.E. Volume 2, The
    2 CD's. Silver Age Classics series. Limited edition of 3,000 copies.
  4. Man From U.N.C.L.E., The (Film Score Monthly FSMCD Vol. 7 No. 14)
    Original Release Title: Man From U.N.C.L.E. Volume 3, The
    Silver Age Classics series. 2 CD's. Limited edition of 3,000 copies.
  5. Girl From U.N.C.L.E., The (Film Score Monthly FSMCD Vol. 7 No. 14)
    Original Release Title: Man From U.N.C.L.E. Volume 3, The
    Silver Age Classics series. 2 CD's. Limited edition of 3,000 copies.
  6. Man From U.N.C.L.E., The (RCA Victor LPM-3574)
    Original Release Title: More Music From The Man From U.N.C.L.E.
    Mono.